We demonstrate high-temperature thermoelectric conversion in InAs/InP nanowire quantum dots by taking advantage of their strong electronic confinement. The electrical conductance G and the thermopower S are obtained from charge transport measurements and accurately reproduced with a theoretical model accounting for the multilevel structure of the quantum dot. Notably, our analysis does not rely on the estimate of cotunnelling contributions, since electronic thermal transport is dominated by multilevel heat transport. By taking into account two spin-degenerate energy levels we are able to evaluate the electronic thermal conductance K and investigate the evolution of the electronic figure of merit ZT as a function of the quantum dot configuration and demonstrate ZT ≈ 35 at 30 K, corresponding to an electronic efficiency at maximum power close to the Curzon-Ahlborn limit.

Thermoelectric Conversion at 30 K in InAs/InP Nanowire Quantum Dots

Prete D.;Erdman P. A.;Demontis V.;Ercolani D.;Beltram F.;Rossella F.;Roddaro S.
2019

Abstract

We demonstrate high-temperature thermoelectric conversion in InAs/InP nanowire quantum dots by taking advantage of their strong electronic confinement. The electrical conductance G and the thermopower S are obtained from charge transport measurements and accurately reproduced with a theoretical model accounting for the multilevel structure of the quantum dot. Notably, our analysis does not rely on the estimate of cotunnelling contributions, since electronic thermal transport is dominated by multilevel heat transport. By taking into account two spin-degenerate energy levels we are able to evaluate the electronic thermal conductance K and investigate the evolution of the electronic figure of merit ZT as a function of the quantum dot configuration and demonstrate ZT ≈ 35 at 30 K, corresponding to an electronic efficiency at maximum power close to the Curzon-Ahlborn limit.
2019
Settore FIS/03 - Fisica della Materia
mesoscopic transport; nanowire; quantum dot; Seebeck effect; Thermoelectric conversion
File in questo prodotto:
File Dimensione Formato  
acs.nanolett.9b00276.pdf

Accesso chiuso

Descrizione: Articolo principale
Tipologia: Published version
Licenza: Non pubblico
Dimensione 3.2 MB
Formato Adobe PDF
3.2 MB Adobe PDF   Richiedi una copia
1903.06935.pdf

accesso aperto

Tipologia: Submitted version (pre-print)
Licenza: Solo Lettura
Dimensione 2.63 MB
Formato Adobe PDF
2.63 MB Adobe PDF

I documenti in IRIS sono protetti da copyright e tutti i diritti sono riservati, salvo diversa indicazione.

Utilizza questo identificativo per citare o creare un link a questo documento: https://hdl.handle.net/11384/81807
Citazioni
  • ???jsp.display-item.citation.pmc??? ND
  • Scopus 62
  • ???jsp.display-item.citation.isi??? 61
  • OpenAlex ND
social impact